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Simon Elliot Wall


Keywords

  • Condensed matter physics
  • Quantum and nanoscale materials
  • Structural dynamics
  • Light induced phase transitions
  • X-ray lasers
  • Synchrotron radiation
  • Symmetry

Head of the Ultrafast Dynamics of Quantum Materials group

Associate Professor

PhD in Physics

Optically controlling quantum materials.

Quantum materials exhibit fascinating and desirable properties, such as high temperature superconductivity, but are challenging to understand. They are complex systems in which multiple degrees of freedom compete to dictate the material’s properties These interactions both make it difficult to understand what drives the emergence of specific properties, but also opens new routes to control their properties.

Our research group exploits the entire electromagnetic spectrum, from THz radiation up to hard X-rays to manipulate and measure the properties of quantum materials. We are particularly interested in how lights can perturb and induce symmetry changes in quantum materials, and how these can be used to manipulate the properties of quantum materials. We do this with a range of lab-based ultrafast optical methods to track materials on timescale of a few femtoseconds and in addition, we exploit newly emerging X-ray lasers to capture atomic and nanoscopic changes in materials with light.

Recent publications

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Rodriguez-Suné, L., Scalora, M., Johnson, A. S., Cojocaru, C., Akozbek, N., Coppens, Z. J., Perez-Salinas, D., Wall, S. & Trull, J. (2020). Second harmonic generation from an ITO nanolayer: Experiment versus theory. In D. L. Andrews, A. J. Bain, M. Kauranen & J.-M. Nunzi (Eds.), Nanophotonics VIII Article 113451R SPIE - International Society for Optical Engineering. https://doi.org/10.1117/12.2555393
Rodríguez-Suné, L., Scalora, M., Johnson, A. S., Cojocaru, C., Akozbek, N., Coppens, Z. J., Perez-Salinas, D., Wall, S. & Trull, J. (2020). Study of second and third harmonic generation from an indium tin oxide nanolayer: Influence of nonlocal effects and hot electrons. APL Photonics, 5(1), Article 010801. https://doi.org/10.1063/1.5129627
Tanikawa, T., Karabekyan, S., Kovalev, S., Casalbuoni, S., Asgekar, V., Bonetti, S., Wall, S., Laarmann, T., Turchinovich, D., Zalden, P., Kampfrath, T., Fisher, A. S., Stojanovic, N., Gensch, M. & Geloni, G. (2020). Volt-per-Ångstrom terahertz fields from X-ray free-electron lasers. Journal of Synchrotron Radiation, 27, 796-798. https://doi.org/10.1107/S1600577520004245
Buades, B., Leon, I., Di Palo, N., Rivas, D. E., Sidiropolous, T. P. H., Severino, S., Reduzzi, M., Cousin, S. L., Hemmer, M., Cocchi, C., Pellegrin, E., Martin, J. H., Manas-Valero, S., Coronado, E., Danz, T., Draxl, C., Uemoto, M., Yabana, K., Schultze, M. ... Biegert, J. (2019). Attosecond soft-X-ray spectroscopy in a transition metal dichalcogenide. In 2019 Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC) IEEE. https://doi.org/10.1109/CLEOE-EQEC.2019.8872837
Ramos-Alvarez, A., Fleischmann, N., Vidas, L., Fernandez-Rodriguez, A., Palau, A. & Wall, S. (2019). Probing the lattice anharmonicity of superconducting YBa2Cu3 O7-δ via phonon harmonics. Physical Review B, 100(18), Article 184302. https://doi.org/10.1103/PhysRevB.100.184302